draw现在分词-我的数学老师作文
Introduction很多文献已经讨论过了
A. Solar
energy conversion by photoelectrochemical cells
has been intensively
investigated. (Nature
1991, 353, 737 - 740 )
B. This was
demonstrated in a number of studies that showed
that composite
plasmonic-metalsemiconductor
photocatalysts achieved significantly higher rates
in
various photocatalytic reactions compared
with their pure semiconductor
counterparts.
C. Several excellent reviews describing these
applications are available, and we do
not
discuss these topics
D. Much work so far has
focused on wide band gap semiconductors for water
splitting for the sake of chemical
stability.(DOI:10.1038NMAT3151)
E. Recent
developments of Lewis acids and water-soluble
organometallic
catalysts have attracted much
attention.(Chem. Rev. 2002, 102, 3641?3666)
F.
An interesting approach in the use of zeolite as a
water-tolerant solid acid was
described by
Ogawa et al(. 2002, 102, 3641?3666)
G.
Considerable research efforts have been devoted to
the direct transition
metal-catalyzed
conversion of aryl halides toaryl nitriles. (J.
Org. Chem. 2000, 65,
7984-7989)
H. There
are many excellent reviews in the literature
dealing with the basic
concepts of the
photocatalytic processand the reader is referred
in particular to those
by Hoffmann and
coworkers,Mills and coworkers, and Kamat.(Metal
oxide
catalysis,19,P755)
I. Nishimiya and
Tsutsumi have reported on(proposed)the influence
of the SiAl
ratio of various zeolites on the
acid strength, which were estimated by calorimetry
using ammonia. (. 2002, 102, 3641?3666)
二、在results and discussion中经常会用到的:如图所示
A.
GIXRD patterns in Figure 1A show the bulk
structural information on
as-deposited films.
B. As shown in Figure 7B, the steady-
state current density decreases after cycling
between 0.35 and 0.7 V, which is probably due
to the dissolution of FeOx.
C. As can be seen
from parts a and b of Figure 7, the reaction
cycles start with the
thermodynamically most
favorable VOx structures(J. Phys. Chem. C 2014,
118,
24950?24958)
这与XX能够相互印证:
A.
This is supported by the appearance in the Ni-
doped compounds of an
ultraviolet–visible
absorption band at 420–520nm (see Fig. 3 inset),
corresponding to
an energy range of about 2.9
to 2.3 eV.
B. This is consistent with the
observation from SEM–EDS. ( et al.
Chemical
Physics Letters 332 (2000) 271–277)
C. This
indicates a good agreement between the observed
and calculated intensities
in monoclinic with
space groupP2c when the O atoms are included in
the model.
D. The results are in good
consistent with the observed photocatalytic
activity...
E. Identical conclusions were
obtained in studies where the SPR intensity and
wavelength were modulated by manipulating the
composition, shape,or size of
plasmonic
nanostructures.
F. It was also found that
areas of persistent divergent surface
flow
coincide with regions where convection appears to
be consistently suppressed
even when SSTs are
above 27.5°C.
1. 值得注意的是...
A. It must
also be mentioned that the recycling of aqueous
organic solvent is less
desirable than that of
pure organic liquid.
B. Another interesting
finding is that zeolites with 10-membered ring
pores showed
high selectivities (>99%) to
cyclohexanol, whereas those with 12-membered ring
pores, such as mordenite, produced large
amounts of dicyclohexyl ether. (Chem. Rev.
2002, 102, 3641?3666)
C. It should
be pointed out that the nanometer-scale
distribution of electrocatalyst
centers on the
electrode surface is also a predominant factor for
high ORR
electrocatalytic activity.
D.
Notably, the Ru II and Rh I complexes possessing
the same BINAP chirality form
antipodal amino
acids as the predominant products. (Angew. Chem.
Int. Ed., 2002, 41:
2008–2022)
E. Given
the multitude of various transformations
published, it is noteworthy that only
very few
distinct activation methods have been identified.
(Chem. Soc. Rev., 2009, 38,
2178-2189)
F.
It is important to highlight that these two
directing effects will lead to different
enantiomers of the products even if both the
“H-bond-catalyst” and the catalyst acting
by
steric shielding have the same absolute
stereochemistry. (Chem. Soc.
Rev., 2009, 38,
2178-2189)
G. It is worthwhile mentioning that
these PPNDs can be very stable for several
months without the observations of any
floating or precipitated dots, which is
attributed to the electrostatic repulsions
between the positively charge PPNDs
resulting
in electrosteric stabilization.(Adv. Mater., 2012,
24: 2037–2041)
2. ...仍然是个挑战
A. There
is thereby an urgent need but it is still a
significant challenge to rationally
design and
delicately tail or the electroactive MTMOs for
advanced LIBs, ECs,
MOBs, and FCs. (Angew.
Chem. Int. Ed.2 014, 53, 1488 – 1504)
B.
However, systems that are sufficiently stable and
efficient for practical use have
not yet been
realized.
C. It remains challenging to
develop highly active HER catalysts based on
materials
that are more abundant at lower
costs. (J. Am. Chem. Soc., 2011, 133, 7296–7299)
D. One of the great challenges in the twenty-
first century is unquestionably energy
storage. (Nature Materials 2005, 4, 366 - 377
)
3. 众所周知
A. It is well
established (accepted) It is known to all It is
commonly
known that many characteristics of
functional materials, such as composition,
crystalline phase, structural and
morphological features, and the sur-interface
properties between the electrode and
electrolyte, would greatly influence the
performance of these unique MTMOs in
electrochemical energy storageconversion
applications.(Angew. Chem. Int. Ed.2014,53,
1488 – 1504)
B. It is generally accepted
(believed) that for a-Fe2O3-based sensors the
change in
resistance is mainly caused by the
adsorption and desorption of gases on the surface
of the sensor structure. (Adv. Mater. 2005,
17, 582)
C. As we all know, soybean abounds
with carbon, nitrogen and oxygen elements
owing to the existence of sugar, proteins and
lipids. (Chem. Commun., 2012, 48,
9367-9369)
D. There is no denying that their presence may
mediate spin moments to align parallel
without
acting alone to show d0-FM. (Nanoscale, 2013, 5,
3918-3930)
1. 正如下文将提到的...
A. As will
be described below(也可以是As we shall see below), as
the SiAl ratio
increases, the surface of the
zeolite becomes more hydrophobic and possesses
stronger affinity for ethyl acetate and the
number of acid sites decreases.(Chem. Rev.
2002, 102, 3641?3666)
B. This behavior is
to be expected and will be further discussed
below. (J. Am. Chem.
Soc., 1955, 77,
3701–3707)
C. There are also some small
deviations with respect to the flow direction,
which
we will discuss below.(Science, 2001,
291, 630-633)
D. Below, we will see what this
implies.
E. Complete details of this case will
be provided at a later time.
E.
很多论文中,也经常直接用see below来表示,比如:The observation of
nanocluster spheres at the ends of the
nanowires is suggestive of a VLS growth
process (see below). (Science, 1998, 279,
208-211)
3. 我们的研究可能在哪些方面得到应用
A. Our
?ndings suggest that the use of solar energy for
photocatalytic water
splitting might provide a
viable source for ?clean? hydrogen fuel, once the
catalytic
ef?ciency of the semiconductor
system has been improved by increasing its surface
area and suitable modi?cations of the surface
sites.
B. Along with this green and cost-
effective protocol of synthesis, we expect that
these
novel carbon nanodots have potential
applications in bioimaging and
electrocatalysis.(Chem. Commun., 2012, 48,
9367-9369)
C. This system could potentially be
applied as the gain medium of solid-state
organic-based lasers or as a component of high
value photovoltaic (PV) materials,
where
destructive high energy UV radiation would be
converted to useful low energy
NIR radiation.
(Chem. Soc. Rev., 2013, 42, 29-43)
D. Since
the use of graphene may enhance the photocatalytic
properties of TiO2 under
UV and visible-light
irradiation, graphene–TiO2 composites may
potentially be used
to enhance the
bactericidal activity. (Chem. Soc. Rev., 2012, 41,
782-796)
E. It is the first report that CQDs
are both amino-functionalized and highly
fluorescent, which suggests their promising
applications in chemical sensing.(Carbon,
2012, 50, 2810–2815)
1. 什么东西还尚未发现系统研究
A. However,systems that are sufficiently
stable and efficient for practical use have not
yet been realized.
B.
Nevertheless,for conventional nanostructured MTMOs
as mentioned above, some
problematic
disadvantages cannot be overlooked.(Angew. Chem.
Int. Ed.2014,53,
1488 – 1504)
C. There are
relatively few studies devoted to determination of
cmc values for block
copolymer micelles.
(Macromolecules 1991, 24, 1033-1040)
D. This
might be the reason why, despite of the great
influence of the preparation on
the catalytic
activity of gold catalysts, no systematic study
concerning the synthesis
conditions has been
published yet. (Applied Catalysis A: General
2002, 226, 1–13)
E. These possibilities
remain to be explored.
F. Further effort is
required to understand and better control the
parameters
dominating the particle surface
passivation and resulting properties for carbon
dots of
brighter photoluminescence. (J. Am.
Chem. Soc., 2006, 128 , 7756–7757)
2.
由于因为...
A. Liquid ammonia is particularly
attractive as an alternative to water due to its
stability in the presence of strong reducing
agents such as alkali metals that are used
to
access lower oxidation states.
B. The unique
nature of the cyanide ligand results from its
ability to act both as a σ
donor and a π
acceptor combined with its negativecharge and
ambidentate nature.
C. Qdots are also
excellent probes for two-photon confocal
microscopy because they
are characterized by a
very large absorption cross section (Science
2005, 307,
538-544).
D. As a result of the
reductive strategy we used and of the strong
bonding between the
surface and the aryl
groups, low residual currents (similar to those
observed at a bare
electrode) were obtained
over a large window of potentials, the same as for
the
unmodified parent GC electrode. (J. Am.
Chem. Soc. 1992, 114, 5883-5884)
E. The
small Tafel slope of the defect-rich MoS2
ultrathin nanosheets is advantageous
for
practical applications, since it will lead to a
faster increment of HER rate with
increasing
overpotential.(Adv. Mater., 2013, 25: 5807–5813)
F. Fluorescent carbon-based materials have
drawn increasing attention in recent
years
owing to exceptional advantages such as high
optical absorptivity, chemical
stability,
biocompatibility, and low toxicity.(Angew. Chem.
Int. Ed., 2013, 52:
3953–3957)
G. On the
basis of measurements of the heat of immersion of
water on zeolites,
Tsutsumi etal. claimed that
the surface consists of siloxane bondings and is
hydrophobicin the region of low Al content.
(Chem. Rev. 2002, 102, 3641?3666)
H.
Nanoparticle spatial distributions might have a
large significance for catalyst
stability,
given that metal particle growth is a relevant
deactivation mechanism for
commercial
catalysts.
3. ...很重要
A. The
inhibition of additional nucleation during growth,
in other words, the complete
separation of
nucleation and growth, is critical(essential,
important) for the successful
synthesis of
monodisperse nanocrystals. (Nature Materials 3,
891 - 895 (2004))
B. In the current study,
Cys, homocysteine (Hcy) and glutathione (GSH) were
chosen
as model thiol compounds since they
play important (significant, vital, critical)
roles in many biological processes and
monitoring of these thiol compounds is of
great importance for diagnosis of
diseases.(Chem. Commun., 2012, 48, 1147-1149)
C. This is because according to nucleation
theory, what really matters in addition to
the
change in temperature ΔT (or supersaturation) is
the cooling rate.(Chem. Soc. Rev.,
2014, 43,
2013-2026)
1. 相反不同于
A. On the
contrary, mononuclear complexes, called single-ion
magnets (SIM), have
shown hysteresis loops of
butterflyphonon bottleneck type, with negligible
coercivity,
and therefore with much
shorter relaxation times of magnetization. (Angew.
Chem.
Int. Ed., 2014, 53: 4413–4417)
B. In
contrast, the Dy compound has significantly larger
value of the transversal
magnetic moment
already in the ground state (ca. 10
?1
μ
B
), therefore allowing a fast
QTM.
(Angew. Chem. Int. Ed., 2014, 53: 4413–4417)
C. In contrast to the structural similarity of
these complexes, their magnetic behavior
exhibits strong divergence. (Angew. Chem. Int.
Ed., 2014, 53: 4413–4417)
D. Contrary to other
conducting polymer semiconductors, carbon nitride
is
chemically and thermally stable and does
not rely on complicated device
manufacturing.
(Nature materials, 2009, 8(1): 76-80.)
E.
Unlike the spherical particles they are derived
from that Rayleigh light-scatter in
the blue,
these nanoprisms exhibit scattering in the red,
which could be useful in
developing multicolor
diagnostic labels on the basis not only of
nanoparticle
composition and size but also of
shape. (Science 2001, 294, 1901-1903)
2.
发现,阐明,报道,证实
可供选择的词包括:verify, confirm,
elucidate, identify, define, characterize,
clarify,
establish, ascertain, explain,
observe, illuminate, illustrate,demonstrate, show,
indicate, exhibit, presented, reveal, display,
manifest,suggest, propose, estimate,
prove,
imply, disclose,report, describe,facilitate the
identification of
举例:
A. These stacks
appear as nanorods in the two-dimensional TEM
images, but tilting
experiments confirmthat
they are nanoprisms. (Science 2001, 294,
1901-1903)
B. Note that TEM shows that about
20% of the nanoprisms are truncated. (Science
2001, 294, 1901-1903)
C. Therefore, these
calculations not only allow us to identify the
important features in
the spectrum of the
nanoprisms but also the subtle relation between
particle shape and
the frequency of the bands
that make up their spectra. (Science 2001, 294,
1901-1903)
D. We observed a
decrease in intensity of the characteristic
surface plasmon band in
the ultraviolet-
visible (UV-Vis) spectroscopy for the spherical
particles at λ
max
= 400
nm with a
concomitant growth of three new bands of
λ
max
= 335 (weak), 470
(medium), and
670 nm (strong), respectively. (Science 2001,
294, 1901-1903)
E. In this article, we present
data demonstrating that opiate and nonopiate
analgesia
systems can be selectively activated
by different environmental manipulations
and
describe the neural circuitry involved. (Science
1982, 216, 1185-1192)
F. This suggests that
the cobalt in CoP has a partial positive charge
(δ
+
), while the
phosphorus has a
partial negative charge (δ
?
), implying a
transfer of electron density
from Co to P.
(Angew. Chem., 2014, 126: 6828–6832)
3.
如何指出当前研究的不足
A. Although these inorganic
substructures can exhibit a high density of
functional
groups, such as bridging OH groups,
and the substructures contribute significantly to
the adsorption properties of the
material,surprisingly little attention has been
devoted
to the post-synthetic
functionalization of the inorganic units within
MOFs. (Chem.
Eur. J., 2013, 19: 5533–5536.)
B. Little is known, however, about the
microstructure of this material. (Nature
Materials 2013,12, 554–561)
C. So far,
very little information is available, and only in
the absorber film, not in the
whole
operational devices. (Nano Lett., 2014, 14 (2), pp
888–893)
D. In fact it should be noted that
very little optimisation work has been carried out
on these devices. (Chem. Commun., 2013, 49,
7893-7895)
E. By far the most architectures
have been prepared using a solution processed
perovskite material, yet a few examples have
been reported that have used an
evaporated
perovskite layer. (Adv. Mater., 2014, 27:
1837–1841.)
F. Water balance issues have been
effectively addressed in PEMFC technology
through a large body of work encompassing
imaging, detailed water content and
water
balance measurements, materials optimization and
modeling, but very few of
these activities
have been undertaken for anion exchange membrane
fuel
cells, primarily due to limited
materials availability and device lifetime. (J.
Polym.
Sci. Part B: Polym. Phys., 2013, 51:
1727–1735)
G. However, none of these studies
tested for Th17 memory, a recently identified T
cell that specializes in controlling
extracellular bacterial infections at mucosal
surfaces. (PNAS, 2013, 111, 787–792)
H.
However, uncertainty still remains as to the
mechanism by which Li salt addition
results in
an extension of the cathodic reduction limit.
(Energy Environ. Sci., 2014, 7,
232-250)
I. There have been a number of high profile
cases where failure to identify the most
stable crystal form of a drug has led to
severe formulation problems in manufacture.
(Chem. Soc. Rev., 2014, 43, 2080-2088)
J.
However, these measurements systematically
underestimate the amount of ordered
material.
( Nature Materials 2013, 12, 1038–1044)
1. 取决于
a. This is an important
distinction, as the overall activity of a catalyst
will depend
on the material properties,
synthesis method, and other possible species that
can be
formed during activation. (Nat. Mater.
2017,16,225–229)
b. This quantitative
partitioning was determined by growing crystals of
the 1:1
host–guest complex between
ExBox
4+
and corannulene. (Nat.
Chem.
2014, 6177–178)
c. They suggested that
the Au particle size may be the decisive factor
for achieving
highly active Au catalysts.(Acc.
Chem. Res., 2014, 47, 740–749)
d. Low-
valent late transition-metal catalysis has become
indispensable to chemical
synthesis, but
homogeneous high-valent transition-metal catalysis
is underdeveloped,
mainly owing to the
reactivity of high-valent transition-metal
complexes and the
challenges associated with
synthesizing them. (Nature2015, 517,449–454)
e. The polar effect is a remarkable property
that enables considerably endergonic C–H
abstractions that would not be possible
otherwise. (Nature 2015, 525, 87–90)
f.
Advances in heterogeneous catalysis must rely on
the rational design of new
catalysts. (Nat.
Nanotechnol. 2017, 12, 100–101)
g.
Likely, the origin of the chemoselectivity may be
also closely related to the H
bonding with the
N or O atom of the nitroso moiety, a similar
H-bonding effect is
known in enamine-based
nitroso chemistry. (Angew. Chem. Int. Ed. 2014,
53:
4149–4153)
2. 有很大潜力
a. The
quest for new methodologies to assemble complex
organic molecules continues
to be a great
impetus to research efforts to discover or to
optimize new catalytic
transformations. (Nat.
Chem. 2015,7, 477–482)
b. Nanosized
faujasite (FAU) crystals have great potential as
catalysts or adsorbents
to more efficiently
process present and forthcoming synthetic and
renewable
feedstocks in oil refining,
petrochemistry and fine chemistry. (Nat. Mater.
2015, 14,
447–451)
c. For this
purpose, vibrational spectroscopy has proved
promising and very
useful. (Acc Chem Res.
2015, 48, 407–413.)
d. While a detailed
mechanism remains to be elucidated and there is
room for
improvement in the yields and
selectivities, it should be remarked that
chirality
transfer upon
trifluoromethylation of enantioenriched
allylsilanes was shown. (Top
Catal. 2014, 57:
967. )
e. The future looks bright for the
use of PGMs as catalysts, both on laboratory and
industrial scales, because the preparation of
most kinds of single-atom metal catalyst
is
likely to be straightforward, and because
characterization of such catalysts has
become
easier with the advent of techniques that readily
discriminate single atoms
from small clusters
and nanoparticles. (Nature 2015, 525, 325–326)
f. The unique mesostructure of the
3D-dendritic MSNSs with mesopore channels of
short length and large diameter is supposed to
be the key role in immobilization of
active
and robust heterogeneous catalysts, andit would
have more hopeful prospects
in catalytic
applications. (ACS Appl. Mater. Interfaces, 2015,
7, 17450–17459)
g. Visible-light
photoredox catalysis offers exciting opportunities
to achieve
challenging carbon–carbon bond
formations under mild and ecologically benign
conditions. (Acc. Chem. Res., 2016, 49,
1990–1996)
3. 因此
同义词:Therefore, thus,
consequently, hence, accordingly, so, as a result
这一条比较简单,这里主要讲一下这些词的副词词性和灵活运用。这些词并不总
是以
插入语的形式出现在句子最前面,还可以灵活的出现在句子的各个部分,典
型的如:
a. Therefore, we shift our focus to free
energies, as these are more relevant for a
reaction rate analysis. (Nat. Mater. 2017, 16,
225–229)
b. In general, the morphologies
and thus performance of state-of-the-art donor
polymers are sensitive to the choice of
fullerene and replacing PC71BM with another
C60-based or non-PCBM fullerene
decreases PSC efficiency to 6-7%. (Nature
Communications 2014, 5, 5239)
c. We
hence determine the steady state excitation
density (where excitations can be
free charge
or excitons) to be between 1013 and 1015 cm?3.
(Nature
Communications 2014, 5, 3586 )
可以变形为:Hence, We determine the steady state
excitation density (where
excitations can be
free charge or excitons) to be between 1013 and
1015 cm?3.
1. 为了进一步说明
A. To gain more
insight, we conducted several X-ray, NMR, and
electrochemical
studies. (Acc. Chem. Res.2015,
48, 2813?2821)
B. To further confirm that
phosphorylation of AMPA-R in hippocampal slices
was
catalyzed by CaM-KII,GluR1 was expressed
in HEK-293 cells with or without
CaM-KII.
(Science 1997, 276, 2042-2045)
C. In order to
trace this dynamic development,it is our goal in
this Letter, to describe
the changes in the
properties of such high efficiency Cu(In,Ga)Se2
(CIGS) solar
cells. (Phys. Stat. Sol.(RRL),
2015, 9: 28–31.)
D. To gainachieve a better
understanding of how the immune system responds to
MPDL3280A, the levels of the IL-18
immunostimulatory cytokine and IFN-γ,which
is
stimulated by IL-18, were examined over several
cycles. (Nature 2014, 515,
558–562 )
E. To
further explore this concept, we provide an
example, where patient A
underwent radical
prostatectomy with undetectable postoperative
serum PSA in 2005.
(Nature Reviews Urology
2017, 14,193–194)
F. In order to deeply
investigate the aggregation properties in this
range of
concentrations, we studied these
condary structure of these peptide derivatives by
CD
and FTIR spectroscopies.(Sci Rep. 2016,
6:26638.)
2. 关于,至于
A.
ConcerningAs to adsorbed thiolates onthe (100)
surfaces of all these metals, the
DFT
calculations reveal that they exhibit a better
stability than the respective (111)
faces in
terms of γ,as shown in the corresponding Tables.
(RSC Adv., 2014, 4,
27730-27754)
B. It
should be noted that the additives were not
evaluated with regard to possible
influence on
reactivity or stability to the reaction
conditions. (Nature Chemistry 2013,
5,
597–601)
C. In the following, we will use
this asymptotic notation also when referring to
the
dimer plasmons for small
separations,although the dimer plasmons in that
case
contain contributions from all
angularmomenta. (Nano Letters, 2004, 4,899–903)
D. Conversely, information regarding the
magnetoelectric coefficients based on
electrical or optical experiments can aid the
determination of magnetic point group
symmetries.
E. The arrival of
nanomaterials gave lithium-ion batteries a new
lease of life and
provided benefits in terms
of capacity, power, cost and materials
sustainability that
are still far from being
fully exploited. (Nature 2008, 451, 652-657)
F. The dominance of the Auger effect in
nanocrystal QDs also implies that even
relatively poorly passivated samples could
behave as well as the best samples when it
comes to gain and stimulated emission, because
as long as trapping rates are lower
than Auger
rates, the twoe-h pair lifetime is determined by
the intrinsic Auger decay.
(Science 2000, 290,
314-317)
3. 然而
However, nevertheless,
nonetheless, on the contrary, in contrast, yet,
even so, but
同样,使用这些词时注意它们的词性,实际上它们也可以灵活运用到句子当中
A.
Nevertheless, because the Auger time scale is
substantially faster than surface
trapping in
these dots, both types of samples showed similar
gain properties.
( Science 2000, 290,
314-317)
B. The existence of optical
gain, however, does not guarantee the development
of
stimulated emission. (Science 2000, 290,
314-317)
C. Even so, the anions may be helping
topre-organise 4, or the Hofmeister anion
effects may be the only effects. (Nature
Chemistry 2009, 1, 403 - 408)